By varying current-loss circuit parameters, the Mach2-tabular collisional radiative equilibrium 2-D radiation magnetohydrodynamic model was tuned to reproduce the radiative and electrical properties of three recent argon gas-puff experiments (same initial conditions) performed on the Z machine at Sandia National Laboratories. The model indicates that there were current losses occurring near or within the diode region of the Z machine during the stagnation phase of the implosion. The 'good' simulation reproduces the experimental K-shell powers, K-shell yields, total powers, percentage of emission radiated in α lines, size of the K-shell emission region, and the average electron temperature near the time-of-peak K-shell power. The calculated atomic populations, ion temperatures, and radial velocities are used as input to a detailed multifrequency ray-trace radiation transport model that includes the Doppler effect. This model is employed to construct time-, space-, and energy-resolved synthetic spectra. The role the Doppler effect likely plays in the experiments is demonstrated by comparing synthetic spectra generated with and without this effect.
Argon gas puffs have produced 330kJ ± 9% of x-ray radiation above 3keV photon energy in fast z-pinch implosions, with remarkably reproducible K-shell spectra and power pulses. This reproducibility in x-ray production is particularly significant in light of the variations in instability evolution observed between experiments. Soft x-ray power measurements and K-shell line ratios from a time-resolved spectrum at peak x-ray power suggest that plasma gradients in these high-mass pinches may limit the K-shell radiating mass, K-shell power, and K-shell yield from high-current gas puffs.
This report summarizes the work completed under the Laboratory Directed Research and Development (LDRD) project 10-0973 of the same title. Understanding the molecular origin of the no-slip boundary condition remains vitally important for understanding molecular transport in biological, environmental and energy-related processes, with broad technological implications. Moreover, the viscoelastic properties of fluids in nanoconfinement or near surfaces are not well-understood. We have critically reviewed progress in this area, evaluated key experimental and theoretical methods, and made unique and important discoveries addressing these and related scientific questions. Thematically, the discoveries include insight into the orientation of water molecules on metal surfaces, the premelting of ice, the nucleation of water and alcohol vapors between surface asperities and the lubricity of these molecules when confined inside nanopores, the influence of water nucleation on adhesion to salts and silicates, and the growth and superplasticity of NaCl nanowires.