Publications

Renewed interest in the development of molten salt reactors has created the need for analytical tools that can perform safeguards assessments on these advanced reactors. This work outlines a flexible framework to perform safeguards analyses on a wide range of advanced reactor designs. The framework consists of two parts, a process model and a safeguards tool. The process model, developed in MATLAB Simulink, simulates the flow materials through a reactor facility. These models are linked to SCALE/TRITON and SCALE/ORIGEN to approximate depletion and decay of fuel salts but are flexible enough to accommodate higher fidelity tools if needed. The safeguards tool uses the process data to calculate common statistical quantities of interest such as material unaccounted for (MUF) and Page's trend test on the standardized independent transformed MUF (SITMUF). This paper documents the development of these tools.

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The Material Protection, Accounting, and Control Technologies (MPACT) program is working toward a 2020 demonstration of Safeguards and Security by Design for advanced fuel cycle facilities. This milestone ties together modeling and experimental work and will initially demonstrate the concept for electrochemical processing facilities. The safeguards modeling tool used is the Separation and Safeguards Performance Model (SSPM). This report outlines the baseline model design that will be used for the 2020 milestone analysis, which was updated to represent a new baseline flowsheet developed for the MPACT program. The model was also used to generate simulation data for other labs to use as part of their safeguards analysis. Finally, this report describes how the 2020 milestone will be met. ACKNOWLEDGEMENTS This work was funded by the Materials Protection, Accounting, and Control Technologies (MPACT) working group as part of the Nuclear Technology Research and Development Program under the U.S. Department of Energy, Office of Nuclear Energy.

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This work describes the ongoing work to develop a molten salt reactor (MSR) model and associated tools for safeguards analysis. A new flowsheet was developed in collaboration with Oak Ridge National Laboratory (ORNL) for the Molten Salt Demonstration Reactor (MSDR). This design was chosen by ORNL as a generic baseline design that could be used for safeguards research. The model has simple chemical processing that is less extensive than the two-fluid flowsheet developed in the last year. A detailed TRITON reactor physics model, provided by ORNL, was implemented into the process model. The process model now includes reactor parameters such as K-eff and decay heat, which could be used as part of an advanced safeguards approach. Finally, a set of generic safeguards tools based on current safeguards approaches were developed. These tools are flexible and can be used with most MSR flowsheets. ACKNOWLEDGEMENTS This work was funded by the Materials Protection Accounting and Control Technologies (MPACT) working group as part of the Fuel Cycle Technologies Program under the U.S. Department of Energy, Office of Nuclear Energy. The authors would also like to acknowledge Ben Betz ler for his work on the reactor physics models that were incorporated into the work and the continued collaboration with ORNL staff.

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Nuclear facilities in the U.S. and around the world face increasing challenges in meeting evolving physical security requirements while keeping costs reasonable. The addition of security features after a facility has been designed and without attention to optimization (the approach of the past) can easily lead to cost overruns. Instead, security should be considered at the beginning of the design process in order to provide robust, yet efficient physical security designs. The purpose of this work is to demonstrate how modeling and simulation can be used to optimize the design of physical protection systems. A suite of tools, including Scribe3D and Blender, were used to model up a generic electrochemical reprocessing facility. Physical protection elements such as sensors, portal monitors, barriers, and guard forces were added to the model based on best practices for physical security. One outsider theft scenario was examined with 4-8 adversaries to determine security metrics. This work fits into a larger Virtual Test Bed 2020 Milestone in the Material Protection, Accounting, and Control Technologies (MPACT) program through the Department of Energy (DOE). The purpose of the milestone is to demonstrate how a series of experimental and modeling capabilities across the DOE complex provide the capabilities to demonstrate complete Safeguards and Security by Design (SSBD) for nuclear facilities. ACKNOWLEDGEMENTS This work was funded by the Materials Protection, Accounting, and Control Technologies (MPACT) working group as part of the Nuclear Technology Research and Development Program under the U.S. Department of Energy, Office of Nuclear Energy.

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The Co-Decontamination (CoDCon) Demonstration experiment at Pacific Northwest National Laboratory (PNNL) is designed to test the separation of a mixed U and Pu product from dissolved spent nuclear fuel. The primary purpose of the project is to demonstrate control of the Pu/U ratio throughout the entire process without producing a pure Pu stream. In addition, the project is quantifying the accuracy and precision to which a Pu/U mass ratio can be achieved. The system includes an on-line monitoring system using spectroscopy to monitor the ratios throughout the process. A dynamic model of the CoDCon flowsheet and the on-line monitoring system was developed to augment the experimental work. This model is based in MATLAB Simulink and provides the ability to expand the range of scenarios that can be examined for process control and determine overall measurement uncertainty. Experimental results have been used to inform and benchmark the model so that it can accurately simulate various transient scenarios. The results of the experimental benchmarking are presented here along with modeled scenarios to demonstrate the control and process monitoring of the system.

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