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Strength of porous α-SiO2in a shock loaded environment: Calibration via Richtmyer-Meshkov instability and validation via Mach lens

Journal of Applied Physics

Hudspeth, Matthew; Olles, Joseph; Mandal, Anirban; Williams, James R.; Root, Seth R.; Vogler, Tracy V.

The strength of brittle porous media is of concern in numerous applications, for example, earth penetration, crater formation, and blast loading. Thus, it is of importance to possess techniques that allow for constitutive model calibration within the laboratory setting. The goal of the current work is to demonstrate an experimental technique allowing for strength assessment of porous media subjected to shock loading, which can be implemented into pressure-dependent yield surfaces within numerical simulation schemes. As a case study, the deviatoric response of distended α-SiO2 has been captured in a tamped Richtmyer-Meshkov instability (RMI) environment at a pressure regime of 4-10 GPa. Hydrocode simulations were used to interpret RMI experimental data, and a resulting pressure-dependent yield surface akin to the often employed modified Drucker-Prager model was calibrated. Simulations indicate that the resulting jet length generated by the RMI is sensitive to the porous media strength, thereby providing a feasible experimental platform capable of capturing the pressurized granular deviatoric response. Furthermore, in efforts to validate the RMI-calibrated strength model, a set of Mach-lens experiments was performed and simulated with the calibrated pressure-dependent yield surface. Excellent agreement between the resulting Mach-lens length in experiment and simulation provides additional confidence to the RMI yield-surface calibration scheme.

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Mesoscale simulations of melt production in porous metals under shock compression

AIP Conference Proceedings

Demaske, B.; Hudspeth, M.; Mandal, A.; Jensen, B.; Crum, R.; Vogler, Tracy V.

Mesoscale simulations of a LiF impactor colliding with a PMMA capsule containing aluminum powder (r00 = 1.5 g/cc) have been performed to investigate shock-induced melting in porous metals. Impact velocities of 1-2.5 km/s are chosen to coincide with in situ X-ray diffraction experiments, which provide direct evidence of shock-induced melting in aluminum powders. Mesoscale simulations show shock heating within the powder is highly nonuniform and melting remains incomplete over hundreds of nanoseconds behind the shock front despite equilibrium pressure-temperature states from continuum simulations lying above the experimental melt line. Such incomplete melting behavior is consistent with X-ray diffraction data obtained in experiment. For an impact velocity of ~1 km/s, mesoscale simulations predict re-solidification behind the shock front as high-temperature regions are cooled below the melt line. Reducing the grain size of the powder by a factor of two leads to a reduction in the time required to reach complete melt such that total melting of the powder may be observed experimentally for an impact velocity of 2.42 km/s.

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Imaging perturbed shock propagation in powders

Review of Scientific Instruments

Cooper, Marcia A.; Sapp, Adam W.; Guo, Shuyue G.; Vogler, Tracy V.

A novel experimental methodology is presented to study the deviatoric response of powders in shock regimes. The powders are confined to a cylindrical wedge volume, and a projectile-driven shock wave with a sinusoidally varying front propagates through the powder. The perturbed shock wave exhibits a damping behavior due to irreversible processes of viscosity and strength (deviatoric) of the powder with propagation through increasing powder thicknesses. The inclined surface of the wedge is polished and coated to establish a diffuse surface suitable for reflecting incident laser light into a high-speed camera imaging at 5 MHz. Images of the contrast loss upon shock wave arrival at the observation surface are post-processed for qualitative and quantitative information. New data of shock damping behavior with parameters of perturbation wavelength and initial shock strength are presented for powders of copper, tantalum, and tungsten carbide as well as their mixtures. We present the first full-field images showing additional spatial disturbances on the perturbed shock front that appear dependent on particle material and morphology.

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Uncertainties in low-pressure shock experiments on heterogeneous materials

Conference Proceedings of the Society for Experimental Mechanics Series

Vogler, Tracy V.; Hudspeth, Matthew; Root, Seth R.

Understanding and quantifying the uncertainties in experimental results are crucial to properly interpreting simulations based on those results. While methods are reasonably well established for estimating those uncertainties in high-pressure shock experiments on homogeneous materials, it is much more difficult to treat relatively low-pressure experiments where shock rise times are significant and material strength is not negligible. Sample heterogeneity further complicates the issue, especially when that heterogeneity is not characterized in each sample. Here, we extend the Monte Carlo impedance matching approach used in high-pressure Z experiments to low-pressure experiments on heterogeneous porous materials. The approach incorporates uncertainties not only in the equation of state of the impedance matching standard but also those associated with its strength. In addition, we also examine approaches for determining material heterogeneity and evaluate its effect on the experimental results.

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Shock compression of strongly correlated oxides: A liquid-regime equation of state for cerium(IV) oxide

Physical Review B

Weck, Philippe F.; Cochrane, Kyle C.; Root, Seth R.; Lane, J.M.; Shulenburger, Luke N.; Carpenter, John H.; Sjostrom, Travis; Mattsson, Thomas M.; Vogler, Tracy V.

The shock Hugoniot for full-density and porous CeO2 was investigated in the liquid regime using ab initio molecular dynamics (AIMD) simulations with Erpenbeck's approach based on the Rankine-Hugoniot jump conditions. The phase space was sampled by carrying out NVT simulations for isotherms between 6000 and 100 000 K and densities ranging from ρ=2.5 to 20g/cm3. The impact of on-site Coulomb interaction corrections +U on the equation of state (EOS) obtained from AIMD simulations was assessed by direct comparison with results from standard density functional theory simulations. Classical molecular dynamics (CMD) simulations were also performed to model atomic-scale shock compression of larger porous CeO2 models. Results from AIMD and CMD compression simulations compare favorably with Z-machine shock data to 525 GPa and gas-gun data to 109 GPa for porous CeO2 samples. Using results from AIMD simulations, an accurate liquid-regime Mie-Grüneisen EOS was built for CeO2. In addition, a revised multiphase SESAME-Type EOS was constrained using AIMD results and experimental data generated in this work. This study demonstrates the necessity of acquiring data in the porous regime to increase the reliability of existing analytical EOS models.

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Trinity Phase 2 Open Science: CTH

Ruggirello, Kevin P.; Vogler, Tracy V.

CTH is an Eulerian hydrocode developed by Sandia National Laboratories (SNL) to solve a wide range of shock wave propagation and material deformation problems. Adaptive mesh refinement is also used to improve efficiency for problems with a wide range of spatial scales. The code has a history of running on a variety of computing platforms ranging from desktops to massively parallel distributed-data systems. For the Trinity Phase 2 Open Science campaign, CTH was used to study mesoscale simulations of the hypervelocity penetration of granular SiC powders. The simulations were compared to experimental data. A scaling study of CTH up to 8192 KNL nodes was also performed, and several improvements were made to the code to improve the scalability.

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Enhanced densification, strength and molecular mechanisms in shock compressed porous silicon

AIP Conference Proceedings

Matthew, J.; Lane, D.; Thompson, Aidan P.; Vogler, Tracy V.

We have recently shown that the final density of silicon under shock compression is anomalously enhanced by introducing voids in the initial uncompressed material. Using molecular simulation, we also demonstrated a molecular mechanism for the effect, which is seen in a growing class of other similar materials. We have shown that this mechanism involves a premature local phase transition nucleated by local shear strain. At higher shock loads we show here that this transition becomes frustrated producing amorphous silicon.We also observe local melting below the equilibrium melt line for bulk silicon. Large-scale non-equilibrium molecular dynamics (NEMD) and Hugoniostat simulations of shock compressed porous silicon are used to study the mechanism. Final stress states and strength were characterized versus initial porosity and for various porosity microstructures.

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Shock Wave Perturbation Decay in Granular Materials

Journal of Dynamic Behavior of Materials

Vogler, Tracy V.

A technique in which the evolution of a perturbation in a shock wave front is monitored as it travels through a sample is applied to granular materials. Although the approach was originally conceived as a way to measure the viscosity of the sample, here it is utilized as a means to probe the deviatoric strength of the material. Initial results for a tungsten carbide powder are presented that demonstrate the approach is viable. Simulations of the experiments using continuum and mesoscale modeling approaches are used to better understand the experiments. The best agreement with the limited experimental data is obtained for the mesoscale model, which has previously been shown to give good agreement with planar impact results. The continuum simulations indicate that the decay of the perturbation is controlled by material strength but is insensitive to the compaction response. Other sensitivities are assessed using the two modeling approaches. The simulations indicate that the configuration used in the preliminary experiments suffers from certain artifacts and should be modified to remove them. The limitations of the current instrumentation are discussed, and possible approaches to improve it are suggested.

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Enhanced densification under shock compression in porous silicon

Physical Review B - Condensed Matter and Materials Physics

Lane, J.M.; Thompson, Aidan P.; Vogler, Tracy V.

Under shock compression, most porous materials exhibit lower densities for a given pressure than that of a full-dense sample of the same material. However, some porous materials exhibit an anomalous, or enhanced, densification under shock compression. We demonstrate a molecular mechanism that drives this behavior. We also present evidence from atomistic simulation that silicon belongs to this anomalous class of materials. Atomistic simulations indicate that local shear strain in the neighborhood of collapsing pores nucleates a local solid-solid phase transformation even when bulk pressures are below the thermodynamic phase transformation pressure. This metastable, local, and partial, solid-solid phase transformation, which accounts for the enhanced densification in silicon, is driven by the local stress state near the void, not equilibrium thermodynamics. This mechanism may also explain the phenomenon in other covalently bonded materials.

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A Nonlocal Peridynamic Plasticity Model for the Dynamic Flow and Fracture of Concrete

Vogler, Tracy V.; Lammi, Christopher J.

A nonlocal, ordinary peridynamic constitutive model is formulated to numerically simulate the pressure-dependent flow and fracture of heterogeneous, quasi-brittle ma- terials, such as concrete. Classical mechanics and traditional computational modeling methods do not accurately model the distributed fracture observed within this family of materials. The peridynamic horizon, or range of influence, provides a characteristic length to the continuum and limits localization of fracture. Scaling laws are derived to relate the parameters of peridynamic constitutive model to the parameters of the classical Drucker-Prager plasticity model. Thermodynamic analysis of associated and non-associated plastic flow is performed. An implicit integration algorithm is formu- lated to calculate the accumulated plastic bond extension and force state. The gov- erning equations are linearized and the simulation of the quasi-static compression of a cylinder is compared to the classical theory. A dissipation-based peridynamic bond failure criteria is implemented to model fracture and the splitting of a concrete cylinder is numerically simulated. Finally, calculation of the impact and spallation of a con- crete structure is performed to assess the suitability of the material and failure models for simulating concrete during dynamic loadings. The peridynamic model is found to accurately simulate the inelastic deformation and fracture behavior of concrete during compression, splitting, and dynamically induced spall. The work expands the types of materials that can be modeled using peridynamics. A multi-scale methodology for simulating concrete to be used in conjunction with the plasticity model is presented. The work was funded by LDRD 158806.

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Density Functional Theory (DFT) simulations of porous tantalum pentoxide

Journal of Physics: Conference Series

Cochrane, K.R.; Vogler, Tracy V.; Desjarlais, Michael P.; Mattsson, Thomas M.

Density Functional Theory (DFT) based molecular dynamics has been established as a method capable of yielding high fidelity results for many materials at a wide range of pressures and temperatures and has recently been applied to complex polymers such as polyethylene, compounds such as ethane or CO2, and oxides such as MgO. We use this method to obtain a Grïneisen Γ and thereby build a Mie-Grüneisen equation of state (EOS) and a Rice-Walsh EOS for tantalum pentoxide (Ta2O5 or tantala) and compare to experimental data. The experimental data have initial densities (ρ00) of approximately 1.13, 3, and 7.4 g/cm 3 reduced from a crystalline of 8.36 g/cm3. We found that r becomes constant at higher temperatures and pressure, but is a function of both density and temperature at lower densities and temperatures. Finally, the Mie-Gruneisen EOS is adequate for modeling the slightly distended Hugoniot with an initial density of 7.4 g/cm3 however it is inadequate for the more porous Hugoniot, while the Rice-Walsh EOS combined with a P-λ crush model approximates the experimental data quite well. © Published under licence by IOP Publishing Ltd.

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Pressure-shear experiments on granular materials

Vogler, Tracy V.; Alexander, Charles S.; Reinhart, William D.

Pressure-shear experiments were performed on granular tungsten carbide and sand using a newly-refurbished slotted barrel gun. The sample is a thin layer of the granular material sandwiched between driver and anvil plates that remain elastic. Because of the obliquity, impact generates both a longitudinal wave, which compresses the sample, and a shear wave that probes the strength of the sample. Laser velocity interferometry is employed to measure the velocity history of the free surface of the anvil. Since the driver and anvil remain elastic, analysis of the results is, in principal, straightforward. Experiments were performed at pressures up to nearly 2 GPa using titanium plates and at higher pressure using zirconium plates. Those done with the titanium plates produced values of shear stress of 0.1-0.2 GPa, with the value increasing with pressure. On the other hand, those experiments conducted with zirconia anvils display results that may be related to slipping at an interface and shear stresses mostly at 0.1 GPa or less. Recovered samples display much greater particle fracture than is observed in planar loading, suggesting that shearing is a very effective mechanism for comminution of the grains.

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High-pressure shock behavior of WC and Ta2O5 powders

Vogler, Tracy V.; Root, Seth R.; Knudson, Marcus D.; Reinhart, William D.

Planar shock experiments were conducted on granular tungsten carbide (WC) and tantalum oxide (Ta{sub 2}O{sub 5}) using the Z machine and a 2-stage gas gun. Additional shock experiments were also conducted on a nearly fully dense form of Ta{sub 2}O{sub 5}. The experiments on WC yield some of the highest pressure results for granular materials obtained to date. Because of the high distention of Ta{sub 2}O{sub 5}, the pressures obtained were significantly lower, but the very high temperatures generated led to large contributions of thermal energy to the material response. These experiments demonstrate that the Z machine can be used to obtain accurate shock data on granular materials. The data on Ta{sub 2}O{sub 5} were utilized in making improvements to the P-{lambda} model for high pressures; the model is found to capture the results not only of the Z and gas gun experiments but also those from laser experiments on low density aerogels. The results are also used to illustrate an approach for generating an equation of state using only the limited data coming from nanoindentation. Although the EOS generated in this manner is rather simplistic, for this material it gives reasonably good results.

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Measuring strength at ultrahigh strain rates

Vogler, Tracy V.

The strain rate sensitivity of materials is measured through a combination of quasistatic, Hopkinson bar, and pressure-shear experiments. The pressure-shear technique has largely been limited to strain rates of order 1E6 1/s. Recent advances in laser and magnetically driven ramp loading have made it possible to achieve significantly higher rates, 1E5-1E8 1/s, under uniaxial strain compression. Strength in these experiments can be calculated by comparing the loading response to the hydrostatic (pressure-density) response of the material for the same density and temperature [Fowles, 1961]. This must be done accounting for the heating due to plastic work in the experiments. Experimental uniaxial strain data for aluminum for strain rates up to 1E8 1/s are examined and compared with existing data. The results are consistent with conventional views of the strain rate sensitivity of aluminum. However, when one considers the higher mean stress (pressure) present in the uniaxial strain experiments and, to a lesser extent, the pressure-shear experiments, one finds the material remains rate insensitive to about 1E7 1/s, two orders of magnitude higher than previously thought. Important caveats about determining strength in this manner will be discussed, and recommendations for future work will be made.

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Meso-scale simulation of the shock compression response of equiaxed and needle morphology Al 6061-T6 powders

AIP Conference Proceedings

Fredenburg, David A.; Vogler, Tracy V.; Thadhani, N.N.

With component sizes approaching the mesoscale, conventional size microstructures offer insufficient homogeneity in mechanical properties, forcing microstructures to be reduced to the nanoscale. This work examines the effect of a nanocrystalline surface layer on the dynamic consolidation response of two different morphology Al 6061-T6 powders. Shock-propagation through equiaxed and needle morphology Al 6061-T6 powder beds initially at 73.5 and 75.0% theoretical density, respectively, is simulated at constant particle velocities ranging between 150 and 850 m/s. Shock velocity-particle velocity relationships are determined for powders both with and without the presence of a 2 μm high strength surface layer, which is representative of a nanocrystalline surface layer. Significant deviations in dynamic response are observed with the presence of the surface layer, especially at lower particle velocities. The equation of state (EOS) for both the homogeneous particles and those with a high strength surface layer are found to be best represented by a piecewise EOS. © 2009 American Institute of Physics.

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Expansion into vacuum of a shocked tungsten carbide-epoxy mixture

Vogler, Tracy V.; Reinhart, William D.; Alexander, Charles S.

The behavior of a shocked tungsten carbide / epoxy mixture as it expands into a vacuum has been studied through a combination of experiments and simulations. X-ray radiography of the expanding material as well as the velocity measured for a stood-off witness late are used to understand the physics of the problem. The initial shock causes vaporization of the epoxy matrix, leading to a multi-phase flow situation as the epoxy expands rapidly at around 8 km/s followed by the WC particles moving around 3 km/s. There are also small amounts of WC moving at higher velocities, apparently due to jetting in the sample. These experiments provide important data about the multi-phase flow characteristics of this material.

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Creating bulk nanocrystalline metal

Yang, Pin Y.; Hall, Aaron C.; Vogler, Tracy V.; Gill, David D.

Nanocrystalline and nanostructured materials offer unique microstructure-dependent properties that are superior to coarse-grained materials. These materials have been shown to have very high hardness, strength, and wear resistance. However, most current methods of producing nanostructured materials in weapons-relevant materials create powdered metal that must be consolidated into bulk form to be useful. Conventional consolidation methods are not appropriate due to the need to maintain the nanocrystalline structure. This research investigated new ways of creating nanocrystalline material, new methods of consolidating nanocrystalline material, and an analysis of these different methods of creation and consolidation to evaluate their applicability to mesoscale weapons applications where part features are often under 100 {micro}m wide and the material's microstructure must be very small to give homogeneous properties across the feature.

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Mesoscale and continuum calculations of wave profiles for shock-loaded granular ceramics

AIP Conference Proceedings

Vogler, Tracy V.; Borg, J.P.

Attenuating wave profiles from shock experiments on tungsten carbide powder are compared to calculations from the continuum P-λ model and a 2-D mesoscale model to gain insight into the suitability of the two models. When calibrated, both models accurately capture the Hugoniot response of the powder and the arrival times of unattenuated steady waves. Their amplitudes are more accurately given by the mesoscale model since its reshock states are above the Hugoniot as seen experimentally; the P-λ model, in contrast, reshocks along the Hugoniot. When the attenuating wave is in the range of the Hugoniot data, the models predict attenuation correctly. However, when attenuation falls below the Hugoniot data both models are somewhat inaccurate, and the material response seems to lie between the two models. The final aspect considered is the wave rise time, which is qualitatively correct for the mesoscale model but completely inaccurate for the P-λ model. © 2007 American Institute of Physics.

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Statistics of the Hugoniot elastic limit from line VISAR

AIP Conference Proceedings

Furnish, Michael D.; Vogler, Tracy V.; Alexander, Charles S.; Reinhart, William D.; Trott, Wayne T.; Chhabildas, Lalit C.

Material heterogeneity appears to give rise to variability in the yield behavior of ceramics and metals under shock loading conditions. The line-imaging VISAR provides a way to measure this variability, which may then be quantified by Weibull statistics or other methods. Weibull methods assign a 2-parameter representation of failure phenomena and variability. We have conducted experiments with tantalum (25 and 40 μm grains) and silicon carbide (SiC-N with 5 μm grains). The tantalum HEL variability did not depend systematically on peak stress, grain size or sample thickness, although the previously observed precursor attenuation was present. SiC-N HEL variability within a single shot was approximately half that of single-point variability in a large family of shots; these results are more consistent with sample-to-sample variation than with variability due to changing shot parameters. © 2007 American Institute of Physics.

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Strength measurements on dry Indiana limestone using Ramp loading techniques

AIP Conference Proceedings

Reinhart, William D.; Vogler, Tracy V.; Chhabildas, L.C.

An accurate method for controlling strain rates in dynamic compressions studies involves using the non-linear elastic property of fused silica to transform an initial shock into a ramp wave of known amplitude and duration. Fused silica when placed between a dry Indiana limestone specimen and a projectile produces strain rates in the range of 104/s. Ramp-loading strain rates are higher than what can be produced on Hopkinson bars and lower than what shock experiments attain. The strength determined at the elastic limit under ramp loading compared to Hopkinson bar measurements shows a significant strength increase with increasing strain rate. © 2007 American Institute of Physics.

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Shock response of dry sand

Reinhart, William D.; Chhabildas, Lalit C.; Vogler, Tracy V.

The dynamic compaction of sand was investigated experimentally and computationally to stresses of 1.8 GPa. Experiments have been performed in the powder's partial compaction regime at impact velocities of approximately 0.25, 0.5, and 0.75 km/s. The experiments utilized multiple velocity interferometry probes on the rear surface of a stepped target for an accurate measurement of shock velocity, and an impedance matching technique was used to deduce the shock Hugoniot state. Wave profiles were further examined for estimates of reshock states. Experimental results were used to fit parameters to the P-Lambda model for porous materials. For simple 1-D simulations, the P-Lambda model seems to capture some of the physics behind the compaction process very well, typically predicting the Hugoniot state to within 3%.

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Static and dynamic compaction of ceramic powders

International Journal of Solids and Structures

Vogler, Tracy V.; Lee, Moo Y.; Grady, D.E.

The static and dynamic compaction of ceramic powders was investigated experimentally using a high-pressure friction-compensated press to achieve static stresses of 1.6 GPa and with a novel gas gun setup to stresses of 5.9 GPa for a tungsten carbide powder. Experiments were performed in the partial compaction region to nearly full compaction. The effects of variables including initial density, particle size distribution, particle morphology, and loading path were investigated in the static experiments. Only particle morphology was found to significantly affect the compaction response. Post-test examination of the powder reveals fracture of the grains as well as breaking at particle edges. In dynamic experiments, steady structured compaction waves traveling at very low velocities were observed. The strain rate within the compaction waves was found to scale nearly linearly with the shock stress, in contrast with many fully dense materials where strain rate scales with stress to the fourth power. Similar scaling is found for data from the literature on TiO2 powder. The dynamic response of WC powder is found to be significantly stiffer than the static response, probably because deformation in the dynamic case is confined to the relatively narrow compaction wave front. Comparison of new static powder compaction results with shock data from the literature for SiO2 also reveals a stiffer dynamic response. © 2006 Elsevier Ltd. All rights reserved.

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Dynamic response of shock-loaded multi-component glasses

Alexander, Charles S.; Vogler, Tracy V.; Reinhart, William D.; Chhabildas, Lalit C.

Glass, in various formulations, may be useful as a transparent armor material. Fused quartz (SiO{sub 2}), modified with either B{sub 2}O{sub 3} (13 % wt.) or Na{sub 2}O (15 % wt.), was studied to determine the effect on the dynamic response of the material. Utilizing powder and two-stage light gas guns, plate impact experiments were conducted to determine the effect on strength properties, including the elastic limits and plastic deformation response. Further, the effect of glass modification on known transitions to higher density phases in fused quartz was evaluated. Results of these experiments will be presented and discussed.

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Exploring pulse shaping for Z using graded-density impactors on gas guns (final report for LDRD project 79879)

Kipp, Marlin E.; Reinhart, William D.; Vogler, Tracy V.

While isentropic compression experiment (ICE) techniques have proved useful in deducing the high-pressure compressibility of a wide range of materials, they have encountered difficulties where large-volume phase transitions exist. The present study sought to apply graded-density impactor methods for producing isentropic loading to planar impact experiments to selected such problems. Cerium was chosen due to its 20% compression between 0.7 and 1.0 GPa. A model was constructed based on limited earlier dynamic data, and applied to the design of a suite of experiments. A capability for handling this material was installed. Two experiments were executed using shock/reload techniques with available samples, loading initially to near the gamma-alpha transition, then reloading. As well, two graded-density impactor experiments were conducted with alumina. A method for interpreting ICE data was developed and validated; this uses a wavelet construction for the ramp wave and includes corrections for the ''diffraction'' of wavelets by releases or reloads reflected from the sample/window interface. Alternate methods for constructing graded-density impactors are discussed.

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High-pressure strength measurements under isentropic loading

Vogler, Tracy V.

Recent advances in magnetic loading techniques have permitted quasi-isentropes to be measured to unprecedented levels. However, the relevant equations for planar waves provide no information about transverse stresses, leaving the deviatoric (strength) behavior of an isentropically loaded material unknown. Because materials are much cooler under isentropic loading than under shock loading, they can remain solid and thus retain strength to very high pressures. Thus, to improve our ability to model material behavior under isentropic loading, techniques to measure strength are needed. In this paper, existing techniques for determining high-pressure strength will be discussed along with their limitations. A technique for assessing the strength of isentropically loaded materials will be presented and used to determine the strength of an aluminum alloy using data from the Z machine and gas gun experiments. These results will be compared to existing models for material strength. Finally, limitations of the technique and future work needed will be discussed.

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Hugoniot and strength behavior of silicon carbide

Proposed for publication in the Journal of Applied Physics.

Vogler, Tracy V.; Reinhart, William D.; Chhabildas, Lalit C.

The shock behavior of two varieties of the ceramic silicon carbide was investigated through a series of time-resolved plate impact experiments reaching stresses of over 140 GPa. The Hugoniot data obtained are consistent for the two varieties tested as well as with most data from the literature. Through the use of reshock and release configurations, reloading and unloading responses for the material were found. Analysis of these responses provides a measure of the ceramic's strength behavior as quantified by the shear stress and the strength in the Hugoniot state. While previous strength measurements were limited to stresses of 20-25 GPa, measurements were made to 105 GPa in the current study. The initial unloading response is found to be elastic to stresses as high as 105 GPa, the level at which a solid-to-solid phase transformation is observed. While the unloading response lies significantly below the Hugoniot, the reloading response essentially follows it. This differs significantly from previous results for B{sub 4}C and Al{sub 2}O{sub 3}. The strength of the material increases by about 50% at stresses of 50-75 GPa before falling off somewhat as the phase transformation is approached. Thus, the strength behavior of SiC in planar impact experiments could be characterized as metal-like in character. The previously reported phase transformation at {approx}105 GPa was readily detected by the reshock technique, but it initially eluded detection with traditional shock experiments. This illustrates the utility of the reshock technique for identifying phase transformations. The transformation in SiC was found to occur at about 104 GPa with an associated volume change of about 9%.

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Variability in dynamic properties of tantalum : spall, attenuation and load/unload

Reinhart, William D.; Trott, Wayne T.; Chhabildas, Lalit C.; Vogler, Tracy V.

A suite of impact experiments was conducted to assess spatial and shot-to-shot variability in dynamic properties of tantalum. Samples had a uniform refined {approx}20 micron grain structure with a strong axisymmetric [111] crystallographic texture. Two experiments performed with sapphire windows (stresses of approximately 7 and 12 GPa) clearly showed elastic-plastic loading and slightly hysteretic unloading behavior. An HEL amplitude of 2.8 GPa (corresponding to Y 1.5 GPa) was observed. Free-surface spall experiments showed clear wave attenuation and spallation phenomena. Here, loading stresses were {approx} 12.5 GPa and various ratios of impactor to target thicknesses were used. Spatial and shot-to-shot variability of the spall strength was {+-} 20%, and of the HEL, {+-} 10%. Experiments conducted with smaller diameter flyer plates clearly showed edge effects in the line and point VISAR records, indicating lateral release speeds of roughly 5 km/s.

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Dynamic behavior of boron carbide

Proposed for publication in Journal of Applied Physics.

Vogler, Tracy V.; Vogler, Tracy V.; Reinhart, William D.; Chhabildas, Lalit C.

Boron carbide displays a rich response to dynamic compression that is not well understood. To address poorly understood aspects of behavior, including dynamic strength and the possibility of phase transformations, a series of plate impact experiments was performed that also included reshock and release configurations. Hugoniot data were obtained from the elastic limit (15-18 GPa) to 70 GPa and were found to agree reasonably well with the somewhat limited data in the literature. Using the Hugoniot data, as well as the reshock and release data, the possibility of the existence of one or more phase transitions was examined. There is tantalizing evidence, but at this time no phase transition can be conclusively demonstrated. However, the experimental data are consistent with a phase transition at a shock stress of about 40 GPa, though the volume change associated with it would have to be small. The reshock and release experiments also provide estimates of the shear stress and strength in the shocked state as well as a dynamic mean stress curve for the material. The material supports only a small shear stress in the shocked (Hugoniot) state, but it can support a much larger shear stress when loaded or unloaded from the shocked state. This strength in the shocked state is initially lower than the strength at the elastic limit but increases with pressure to about the same level. Also, the dynamic mean-stress curve estimated from reshock and release differs significantly from the hydrostate constructed from low-pressure data. Finally, a spatially resolved interferometer was used to directly measure spatial variations in particle velocity during the shock event. These spatially resolved measurements are consistent with previous work and suggest a nonuniform failure mode occurring in the material.

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A distributional model for elastic-plastic behavior of shock loaded materials

Vogler, Tracy V.; Vogler, Tracy V.; Asay, James R.

To address known shortcomings of classical metal plasticity for describing material behavior under shock loading, a model which incorporates a distribution in the deviatoric stress state is developed. This distribution will translate in stress space under loading, and growth of the distribution can be included in the model as well. This proposed model is capable of duplicating the key features of a set of reshock and release experiments on 6061-T6 aluminum, many of which are not captured by classical plasticity. The model is relatively simple, is only moderately more computationally intensive, and requires few additional material parameters.

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Tube fragmentation of multiple materials

Vogler, Tracy V.; Thornhill, Tom F.; Chhabildas, Lalit C.; Vogler, Tracy V.

In the current study we are developing an experimental fracture material property test method specific to dynamic fragmentation. This test method allows the study of fracture fragmentation in a reproducible laboratory environment under well-controlled loading conditions. Motion and fragmentation of the specimen are diagnosed using framing camera, VISAR and soft recovery methods. Fragmentation properties of several steels, nitinol, tungsten alloy, copper, aluminum, and titanium have been obtained to date. The values for fragmentation toughness, and failure threshold will be reported, as well as effects in these values as the material strain-rate is varied through changes in wall thickness and impact conditions.

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HVL{_}CTH: A Simple Tool That Simulates The Hyper-Velocity Launch of a Flyer Plate

Vogler, Tracy V.; Vogler, Tracy V.; Chhabildas, Lalit C.

Sandia National Laboratories has developed a unique method for a hyper-velocity launch (HVL), the three-stage gun. The three-stage gun is a modified two-stage light-gas gun, consisting of a piston used in the first stage, an impactor in the second stage, and a flyer plate in the third stage. The impactor is made up of different material layers that are increasing in shock impedance. The graded or pillowed layers allow the flyer to be launched at velocities up to 16 km/s without the formation of a single shock wave in the flyer plate and without it melting. Under certain experimental conditions the flyer velocity cannot be measured by standard means, X-rays and VISAR. Also, there is a need to know the flyer velocity prior to a launch in order to calibrate instruments and determine the appropriate shot configuration. The objective of HVL{_}CTH is to produce an accurate forecast of the flyer plate velocity under different launch conditions. CTH is a Eulerian shock physics computational analysis package developed at Sandia National Laboratories. Using CTH requires knowledge of its syntax and capabilities. HVL{_}CTH allows the user to easily interface with CTH, through the use of Fortran programs and batch files, in order to simulate the three-stage launch of a flyer plate. The program, HVL{_}CTH, requires little to no knowledge of the CTH program and greatly reduces the time needed to calculate the flyer velocity. Users of HVL{_}CTH are assumed to have no experience with CTH. The results from HVL{_}CTH were compared to results of X-ray and VISAR measurements obtained from HVL experiments. The comparisons show that HVL{_}CTH was within 1-2% of the X-Ray and VISAR results most of the time.

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