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A comparison of the neutron detection efficiency and response characteristics of two pixelated PSD-capable organic scintillator detectors with different photo-detection readout methods

Journal of Instrumentation

Marleau, P.; Sweany, Melinda D.; Balajthy, Jon A.

We characterize the performance of two pixelated neutron detectors: a PMT-based array that utilizes Anger logic for pixel identification and a SiPM-based array that employs individual pixel readout. The SiPM-based array offers improved performance over the previously developed PMT-based detector both in terms of uniformity and neutron detection efficiency. Each detector array uses PSD-capable plastic scintillator as a detection medium. We describe the calibration and neutron efficiency measurement of both detectors using a 137Cs source for energy calibration and a 252Cf source for calibration of the neutron response. We find that the intrinsic neutron detection efficiency of the SiPM-based array is (30.2 ± 0.9)%, which is almost twice that of the PMT-based array, which we measure to be (16.9 ± 0.1)%.

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Characterization of ORNL PSD ASIC

Tiano, Elicia K.O.; Sweany, Melinda D.

The performance of the ORNL ASIC and its readout system was tested with pixelated organic scintillators. We use a pixelated trans-Stilbene scintillator array from Inrad Optics and a pixelated organic glass scintillator array developed at Sandia National Laboratories to characterize the energy and timing resolutions and the pulse-shape discrimination (PSD) figure-of-merit (FoM). The results are compared to previous work in which the same metrics were measured on waveforms digitized at 250 MHz with 14-bit resolution. We found that the PSD FoM at 340 keVee of the ASIC configuration compared to waveform data varied with the scintillator type. We measured a PSD FoM of 1.12 ± 0.14 with the ASIC configuration versus 1.39 ± 0.23 with waveform data using the trans-Stilbene array. We measured a PSD FoM of 0.52 ± 0.18 with the ASIC configuration versus 1.25 ± 0.19 with waveform data using the the organic glass scintillator array. The coincidence timing resolution was measured using two 6x6x6 mm3 cubes of trans-Stilbene. It was measured to be 805 ± 9 ps with the ASIC configuration versus 300 ps on average with waveform data.

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ASIC Scoping Study Final Report

Brubaker, E.; Sweany, Melinda D.; Tiano, Elicia K.O.; Becker, Eric; Fabris, Lorenzo; Grace, Carl; Hausladen, Paul A.; Johnson, Jyothis; Matta, James T.; Rescia, Sergio; Rose Jr., Paul B.; Wood, Lynn; Kay, Randolph R.

This report documents the results and findings of a one-year scoping study investigating multichannel readout application specific integrated circuits (ASICs) for interfacing to, and processing data from, silicon photomultiplier (SiPM) arrays. We document ASIC desired and required specifications for four applications supporting national security mission areas: neutron radiography, associated particle imaging, and two versions of kinematic neutron imaging cameras. While each application has a few unique requirements that stress capability, there is generally good agreement among most. Two recently developed ASIC devices were evaluated in a system-like configuration by interfacing these to scintillator crystals exposed to gamma and neutron sources. The 64-channel ORNL device delivered functional capability while meeting most mission requirements for neutron radiography. The Nalu Scientific device, a 32-channel full waveform digitizer, did not demonstrate reliable neutron / gamma separation but it is unclear if this was an ASIC issue or problems with test setup or firmware. A literature survey of other commercial and academic ASICs was undertaken to with the conclusion that existing devices do not meet all requirements.

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Pulse shape measurements for neutron/gamma discrimination using the TOFPET2 ASIC

Journal of Instrumentation

Sweany, Melinda D.; Weinfurther, Kyle J.; Marleau, P.

Many highly pixelated organic scintillator detection systems would benefit from independent readout of each scintillator pixel. Recent advances in Silicon Photomultiplier (SiPM) technology makes this goal feasible, however the data acquisition from potentially hundreds or thousands of channels requires a low-cost and compact solution. For pixelated neutron detection with organic scintillators, the capability to distinguish between neutron and gamma interactions using Pulse Shape Discrimination (PSD) is required along with pulse charge and time of arrival. The TOFPET2 ASIC from PETsys Electronics is a 64-channel readout chip providing pulse time and charge integration measurements from SiPMs, and is specifically designed for time-of-flight positron-emission tomography. Using an 8 × 8 array of 6 mm × 6 mm J-series SiPMs from SensL/OnSemi (ArrayJ-60035-64P-PCB), we have studied the energy and PSD performance of the TOFPET2 ASIC using a 4 × 4 array of 6 mm × 6 mm × 30 mm trans-Stilbene crystals from Inrad Optics and a custom SiPM routing board from PETsys Electronics. Using a time-over-threshold method, we measure a maximum PSD figure-of-merit of approximately 1.2 at 478 keV (the Compton edge of 662 keV) for a J-series SiPM operating at an over-voltage of 3V.

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System Response Characterization for a d–t Neutron Radiography System

Sweany, Melinda D.; Weinfurther, Kyle J.; Sjoberg, Kurt C.; Marleau, P.

We report the system response of a pixelated associated particle imaging (API) neutron radiography system. The detector readout currently consists of a 2x2 array of organic glass scintillator detectors, each with an 8x8 array of optically isolated pixels that match the size and pitch of the ARRAYJ-60035-64P-PCB Silicon Photomultiplier (SiPM) array from SensL/onsemi with 6x6 mm2 SiPMs. The alpha screen of the API deuterium-tritium neutron generator is read out with the S13361-3050AE-08 from Hamamatsu, which is an 8x8 array of 3x3 mm2 SiPMs. Data from the 320 channel system is acquired with the TOFPET2-based readout system. We present the predicted imaging capability of an eventual 5x5 detector array, the waveform-based energy and pulse shape characterization of the individual detectors, and the timing and energy response from the TOFPET2 system.

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Modification of a Silicon Photomultiplier for Reduced High Temperature Dark Count Rate

Balajthy, Jon A.; Burkart, James; Christiansen, Joel T.; Sweany, Melinda D.; Udoni, Darlene; Weber, Thomas M.

In this work we present a novel method for improving the high-temperature performance of silicon photomultipliers (SiPMs) via focused ion beam (FIB) modification of individual microcells. The literature suggests that most of the dark count rate (DCR) in a SiPM is contributed by a small percentage (<5%) of microcells. By using a FIB to electrically deactivate this relatively small number of microcells, we believe we can greatly reduce the overall DCR of the SiPM at the expense of a small reduction in overall photodetection efficiency, thereby improving its high temperature performance. In this report we describe our methods for characterizing the SiPM to determine which individual microcells contribute the most to the DCR, preparing the SiPM for FIB, and modifying the SiPM using the FIB to deactivate the identified microcells.

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Design and Characterization of an Optically Segmented Single Volume Scatter Camera Module

IEEE Transactions on Nuclear Science

Keefe, Kevin; Alhajaji, Hassam; Brubaker, E.; Druetzler, Andrew; Learned, John; Maggi, Paul; Manfredi, Juan J.; Nishimura, Kurtis; Souza, Bejamin P.; Steele, J.; Sweany, Melinda D.; Takahashi, Eric

The optically segmented single volume scatter camera (OS-SVSC) aims to image neutron sources for nuclear nonproliferation applications using the kinematic reconstruction of elastic double-scatter events. We report on the design, construction, and calibration of one module of a new prototype. The module includes 16 EJ-204 organic plastic scintillating bars individually wrapped in Teflon tape, each measuring 0.5 {\mathrm {cm}}\times 0.5 {\mathrm {cm}}\times 20 {\mathrm {cm}}. The scintillator array is coupled to two custom silicon photomultiplier (SiPM) boards consisting of a 2\times 8 array of SensL J-Series-60035 SiPMs, which are read out by a custom 16 channel DRS4 based digitizer board. The electrical crosstalk between SiPMs within the electronics chain is measured as 0.76\% \,\pm \,0.11\% among all 16 channels. We report the detector response of one module including interaction position, time, and energy, using two different optical coupling materials: EJ-560 silicone rubber optical coupling pads and EJ-550 optical coupling grease. We present results in terms of the overall mean and standard deviation of the z -position reconstruction and interaction time resolutions for all 16 bars in the module. We observed the 1\sigma z -position resolution for gamma interactions in the 0.3-0.4 MeVee range to be 2.24 cm ± 1.10 cm and 1.45 cm ± 0.19 cm for silicone optical coupling pad and optical grease, respectively. The observed 1\sigma interaction time resolution is 265 ps ± 29 ps and 235 ps ± 10 ps for silicone optical coupling pad and optical grease, respectively.

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First-principle SiPM Characterization to Enable Radiation Detection in Harsh Environments

2022 IEEE NSS/MIC RTSD - IEEE Nuclear Science Symposium, Medical Imaging Conference and Room Temperature Semiconductor Detector Conference

Fritchie, Jacob W.; Balajthy, Jon A.; Sweany, Melinda D.; Weber, Thomas M.

This paper reports the experimental comparison of two silicon photomultipliers (SiPMs): the MicroFJ-30035 by ONSemi and the ASD-NUV3S-P by AdvanSiD, in terms of gain, dark count rate, and crosstalk probability. SiPMs are solid state photon detectors that enable high sensitivity light readout. They have low-voltage power requirements, small form factor, and are durable. For these reasons, they are being considered as replacements for vacuum photomultiplier tubes in some applications. However, their performance relies on several parameters, which need to be carefully characterized to enable their high-fidelity simulation and SiPM-based design of devices capable to operate in harsh environments. The parameters tend to vary between manufacturers and processing technologies. In this work, we have compared the MicroFJ and ASD SiPMs in terms of gain, dark count rate, and crosstalk probability. We found that the dark count rate of the MicroFJ was 16% higher than the ASD. Also, the gain of the MicroFJ is 3.5 times higher than the ASD. Finally, the crosstalk probability of the ASD 1.96 times higher than the MicroFJ. Our findings are in good agreement with manufacturer reported values.

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Design and calibration of an optically segmented single volume scatter camera for neutron imaging

Journal of Instrumentation

Galindo-Tellez, A.; Keefe, Kevin P.; Adamek, E.; Brubaker, E.; Crow, B.; Dorrill, R.; Druetzler, A.; Felix, C.J.; Kaneshige, N.; Learned, J.G.; Manfredi, J.J.; Nishimura, K.; Souza, B.P.; Schoen, D.; Sweany, Melinda D.

The Optically Segmented Single Volume Scatter Camera (OS-SVSC) aims to image neutron sources for non-proliferation applications using the kinematic reconstruction of elastic double-scatter events. Our prototype system consists of 64 EJ-204 organic plastic scintillator bars, each measuring 5 mm × 5 mm × 200 mm and individually wrapped in Teflon tape. The scintillator array is optically coupled to two silicon photomultiplier ArrayJ-60035 64P-PCB arrays, each comprised of 64 individual 6 mm × 6 mm J-Series sensors arranged in an 8 × 8 array. We report on the design details, including component selections, mechanical design and assembly, and the electronics system. The described design leveraged existing off-the-shelf solutions to support the rapid development of a phase 1 prototype. Several valuable lessons were learned from component and system testing, including those related to the detector’s mechanical structure and electrical crosstalk that we conclude originates in the commercial photodetector arrays and the associated custom breakout cards. We detail our calibration efforts, beginning with calibrations for the electronics, based on the IRS3D application-specific integrated circuits, and their associated timing resolutions, ranging from 30 ps to 90 ps. With electronics calibrations applied, energy and position calibrations were performed for a set of edge bars using 22Na and 90Sr, respectively, reporting an average resolution of (12.07 ± 0.03) mm for energy depositions between 900 keVee and 1000 keVee. We further demonstrate a position calibration method for the internal bars of the matrix using cosmic-ray muons as an alternative to emission sources that cannot easily access these bars, with an average measured resolution of (14.86 ± 0.29) mm for depositions between 900 keVee and 1000 keVee. The coincident time resolution reported between pairs of bars measured up to 400 ps from muon acquisitions. Energy and position calibration values measured with muons are consistent with those obtained using particle emission sources.

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Single Volume Scatter Camera: Optically Segmented Effort - Single Slide Overview

Sweany, Melinda D.; Adamek, E.; Alhajaji, H.; Brown, James R.; Balathy, John; Brubaker, E.; Cabrera-Palmer, B.; Cates, J.C.B.; Dorril, R.; Druetzler, A.; Elam, J.; Febbraro, M.; Feng, Patrick L.; Folsom, Michael W.; Gabella, G.; Galindo-Tellez, A.; Goldblum, B.; Hausladen, P.; Kaneshige, N.; Keffe, Kevin; Laplace, T.A.; Maggi, Paul; Mane, A.; Manfredi, J.; Marleau, P.; Mattingly, J.; Mishra, M.; Moustafa, A.; Nattress, J.; Nishimura, K.; Pinto-Souza, B.; Steele, J.; Takahashi, E.; Ziock, K.

Abstract not provided.

Single Volume Scatter Camera: Optically Segmented Effort

Sweany, Melinda D.; Adamek, E.; Alhajaji, H.; Brown, James R.; Balathy, John; Brubaker, E.; Cabrera-Palmer, B.; Cates, J.C.B.; Dorril, R.; Druetzler, A.; Elam, J.; Febbraro, M.; Feng, Patrick L.; Folsom, Michael W.; Gabella, G.; Galindo-Tellez, A.; Goldblum, B.; Hausladen, P.; Kaneshige, N.; Keffe, Kevin; Laplace, T.A.; Maggi, Paul; Mane, A.; Manfredi, J.; Marleau, P.; Mattingly, J.; Mishra, M.; Moustafa, A.; Nattress, J.; Nishimura, K.; Pinto-Souza, B.; Steele, J.; Takahashi, E.; Ziock, K.

Abstract not provided.

The Single-Volume Scatter Camera

Manfredi, Juan; Adamek, Evan; Brown, Joshua; Brubaker, E.; Cabrera-Palmer, B.; Cates, Joshua; Dorrill, Ryan; Druetzler, Andrew; Elam, Jeff; Feng, Patrick L.; Folsom, Micah; Galindo-Tellez, Aline; Goldblum, Bethany; Hausladen, Paul; Kaneshige, Nathan; Keefe, Kevin P.; Laplace, Thibault; Learned, John; Mane, Anil; Marleau, P.; Mattingly, John; Mishra, Mudit; Moustafa, Ahmed; Nattress, Jason; Steele, J.; Sweany, Melinda D.; Weinfurther, Kyle J.; Ziock, Klaus-Peter

Abstract not provided.

Characterization of a silicon photo-multiplier array with summing board as a photo-multiplier tube replacement in organic scintillator assemblies

Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment

Sweany, Melinda D.; Marleau, P.; Allwork, C.; Kallenbach, G.; Hammon, Steven

We report on the energy, timing, and pulse-shape discrimination performance of cylindrical 5.08 cm diameter × 5.08 cm thick and 7.62 cm diameter × 7.62 cm thick trans-stilbene crystals read out with the passively summed output of three different commercial silicon photo-multiplier arrays. Our results indicate that using the summed output of an 8 × 8 array of SiPMs provides performance competitive with photo-multiplier tubes for many neutron imaging and correlated particle measurements. For a 5.08 cm diameter × 5.08 cm thick crystal read out with SensL's ArrayJ-60035_64P-PCB, which had the best overall properties, we measure the energy resolution as 17.8 ± 0.8% at 341 keVee (σ/E), the timing resolution in the 180–400 keVee range as 236 ± 61 ps (σ), and the pulse-shape discrimination figure-of-merit as 2.21 ± 0.03 in the 230–260 keVee energy range. For a 7.62 cm diameter × 7.62 cm thick crystal read out with SensL's ArrayJ-60035_64P-PCB, we measure the energy resolution as 21.9 ± 2.3% at 341 keVee, the timing resolution in the 180–400 keVee range as 518 ± 42 ps, and the pulse-shape discrimination figure-of-merit as 1.49 ± 0.01 in the 230–260 keVee energy range. These results enable many scintillator-based instruments to enjoy the size, robustness, and power benefits of silicon photo-multiplier arrays as replacement for the photo-multiplier tubes that are predominantly used today.

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The single-volume scatter camera

Proceedings of SPIE - The International Society for Optical Engineering

Manfredi, Juan J.; Adamek, Evan; Brown, Joshua A.; Brubaker, E.; Cabrera-Palmer, B.; Cates, Joshua; Dorrill, Ryan; Druetzler, Andrew; Elam, Jeff; Feng, Patrick L.; Folsom, Micah; Galindo-Tellez, Aline; Goldblum, Bethany L.; Hausladen, Paul; Kaneshige, Nathan; Keefe, Kevin P.; Laplace, Thibault A.; Learned, John G.; Mane, Anil; Marleau, P.; Mattingly, John; Mishra, Mudit; Moustafa, Ahmed; Nattress, Jason; Steele, J.; Sweany, Melinda D.; Weinfurther, Kyle J.; Ziock, Klaus P.

The multi-institution Single-Volume Scatter Camera (SVSC) collaboration led by Sandia National Laboratories (SNL) is developing a compact, high-efficiency double-scatter neutron imaging system. Kinematic emission imaging of fission-energy neutrons can be used to detect, locate, and spatially characterize special nuclear material. Neutron-scatter cameras, analogous to Compton imagers for gamma ray detection, have a wide field of view, good event-by-event angular resolution, and spectral sensitivity. Existing systems, however, suffer from large size and/or poor efficiency. We are developing high-efficiency scatter cameras with small form factors by detecting both neutron scatters in a compact active volume. This effort requires development and characterization of individual system components, namely fast organic scintillators, photodetectors, electronics, and reconstruction algorithms. In this presentation, we will focus on characterization measurements of several SVSC candidate scintillators. The SVSC collaboration is investigating two system concepts: the monolithic design in which isotropically emitted photons are detected on the sides of the volume, and the optically segmented design in which scintillation light is channeled along scintillator bars to segmented photodetector readout. For each of these approaches, we will describe the construction and performance of prototype systems. We will conclude by summarizing lessons learned, comparing and contrasting the two system designs, and outlining plans for the next iteration of prototype design and construction.

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Effect of Teflon Wrapping on the Interaction Position Reconstruction Resolution in Long, Thin Plastic Scintillator Pillars

2020 IEEE Nuclear Science Symposium and Medical Imaging Conference, NSS/MIC 2020

Moustafa, Ahmed; Galindo-Tellez, Aline; Sweany, Melinda D.; Brubaker, E.; Mattingly, John

An optically-segmented single-volume scatter camera is being developed to image MeV-energy neutron sources. The design employs long, thin, optically isolated organic scintillator pillars with 5 mm × 5 mm × 200 mm dimensions (i.e., an aspect-ratio of 1:1:40). Teflon reflector is used to achieve optical isolation and improve light collection. The effect of Teflon on the ability to resolve the radiation interaction locations along such high aspect-ratio pillars is investigated. It was found that reconstruction based on the amplitude of signals collected on both ends of a bare pillar is less precise than reconstruction based on their arrival times. However, this observation is reversed after wrapping in Teflon, such that there is little to no improvement in reconstruction resolution calculated by combining both methods. It may be possible to use another means of optical isolation that does not require wrapping each individual pillar of the camera.

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Position and Timing Resolution Measurements ofOrganic-Glass scintillator bars for the OpticallySegmented Single-Volume Scatter Camera

Sweany, Melinda D.; Brown, Jason; Cabrera-Palmer, B.; Carlson, Joseph; Dorrill, R.; Druetzler, A.; Elam, J.; Febbraro, M.; Feng, Patrick L.; Folsom, Michael W.; Galino-Tellez, A.; Goldblum, B.; Hausladen, P.; Kaneshige, N.; Keffe, K.; Laplace, T.; Learned, J.; Mane, A.; Manfredi, Juan; Marleau, P.; Mattingly, J.; Mishra, M.; Moustafa, A.; Nattress, J.; Steele, J.; Weinfurther, K.; Ziock, K.

Abstract not provided.

Current Status of an Optically-Segmented Single-Volume Scatter Camera for Neutron Imaging

Brown, J.A.; Brubaker, E.; Dorril, R.; Druetzler, A.; Elam, J.; Febbraro, M.; Feng, Patrick L.; Folsom, Michael W.; Galino-Tellez, A.; Goldblum, B.L.; Hausladen, P.; Kaneshige, N.; Keffe, K.; Laplace, T.A.; Learned, J.G.; Mane, A.; Manfredi, J.; Marleau, Peter; Mattingly, J.; Mishra; Almanza-Madrid, Rene A.; Moustafa, A.; Nattress, J.; Steele, J.; Sweany, Melinda D.; Weinfurther, K.; Ziock, K.

Abstract not provided.

Current status of an optically-segmented single-volume scatter camera for neutron imaging

Brown, Joshua; Brubaker, E.; Cabrera-Palmer, B.; Carlson, Joseph; Dorril, Ryan; Druetzler, Andrew; Elam, Jeff; Febbraro, Michael; Feng, Patrick L.; Folsom, Micah; Galino-Tellez, Aline; Goldblum, Bethany; Hausladen, Paul; Kaneshige, Nate; Keffe, Kevin; Laplace, Tibo; Learned, John; Mane, Anil; Manfredi, Juan; Marleau, P.; Mattingly, John; Mishra, Mudit; Moustafa, Ahmed; Nattress, Jason; Nishimura, Kurtis; Steele, J.; Sweany, Melinda D.; Ziock, Klaus

Abstract not provided.

Design and Evaluation of a Pixelated PSD-capable Scintillator Detector with SiPM Readout

Sweany, Melinda D.; Marleau, P.; Hammon, Steven; Kallenbach, Gene; Polack, John K.

We present the detector response comparison between a 10x10 pixellated array of scintillator read out with Anger logic using four 2" Hamamatsu R7724-100 super bialkali photomultiplier tubes (PMT) and a custom Silicon photomultiplier (SiPM) board consisting of 100 C-series 6x6 mm SiPMs from SensL. An array of these pixellated detectors are currently used in the Neutron Coded Aperture (NCA) imaging system. The energy, timing and pulse shape discrimination response using both readout schemes are presented, along with an analysis of multiple scatter events occurring within the block. An evaluation of the impact of photodetector readout on the overall detection efficiency and imaging accuracy is presented.

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Interaction position, time, and energy resolution in organic scintillator bars with dual-ended readout

Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment

Sweany, Melinda D.; Brown, J.; Brubaker, E.; Dorrill, R.; Druetzler, A.; Galindo-Tellez, A.; Kaneshige, N.; Learned, J.; Nishimura, K.; Wonseok, Bae

We report on the position, timing, and energy resolution of a range of plastic scintillator bars and reflector treatments using dual-ended silicon photomultiplier readout. These measurements are motivated by the upcoming construction of an optically segmented single-volume neutron scatter camera, in which neutron elastic scattering off of hydrogen is used to kinematically reconstruct the location and energy of a neutron-emitting source. For this application, interaction position resolutions of about 10 mm and timing resolutions of about 1 ns are necessary to achieve the desired efficiency for fission-energy neutrons. The results presented here indicate that this is achievable with an array of 5×5×190mm 3 bars of EJ-204 scintillator wrapped in Teflon tape, read out with SensL's J-series 6×6mm 2 silicon photomultipliers. With two independent setups, we also explore the systematic variability of the position resolution, and show that, in general, using the difference in the pulse arrival time at the two ends is less susceptible to systematic variation than using the log ratio of the charge amplitude of the two ends. Finally, we measure a bias in the absolute time of interactions as a function of position along the bar: the measured interaction time for events at the center of the bar is ∼100 ps later than interactions near the SiPM.

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Characterization of a Silicon photo-multiplier summing breakout board for photo-multiplier tube replacement

Sweany, Melinda D.; Marleau, P.; Kallenbach, Gene A.

We present the relative timing and pulse-shape discrimination performance of a H1949-50 photomultiplier tube to SensL ArrayX-B0B6_64S coupled to a SensL ArrayC-60035-64P- PCB Silicon Photomultiplier array. The goal of this work is to enable the replacement of photomultiplier readout of scintillators with Silicon Photomultiplier devices, which are more robust and have higher particle detection efficiency. The report quantifies the degradation of these performance parameters using commercial off the shelf summing circuits, and motivates the development of an improved summing circuit: the pulse-shape descrimination figure-of-merit drops from 1.7 at 500 keVee to 1.4, and the timing resolution (σ) is 288 ps for the photomultiplier readout and approximately 1 ns for the Silicon Photomultiplier readout. A degradation of this size will have a large negative impact on any device that relies on timing coincidence or pulse-shape discrimination to detect neutron interactions, such as neutron kinematic imaging or multiplicity measurements.

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Feasibility of Single-sided 3D elemental imaging

Sweany, Melinda D.; Gerling, Mark; Marleau, P.; Monterial, Mateusz

We present single-sided 3D image reconstruction and neutron spectrum of non-nuclear material interrogated with a deuterium-tritium neutron generator. The results presented here are a proof-of-principle of an existing technique previously used for nuclear material, applied to non-nuclear material. While we do see excess signatures over background, they do not have the expected form and are currently un-identified.

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Source detection at 100 meter standoff with a time-encoded imaging system

Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment

Brennan, J.; Brubaker, E.; Gerling, Mark; Marleau, P.; Monterial, M.; Nowack, A.; Schuster, P.; Sturm, B.; Sweany, Melinda D.

We present the design, characterization, and testing of a laboratory prototype radiological search and localization system. The system, based on time-encoded imaging, uses the attenuation signature of neutrons in time, induced by the geometrical layout and motion of the system. We have demonstrated the ability to detect a ∼1mCi252Cf radiological source at 100m standoff with 90% detection efficiency and 10% false positives against background in 12min. This same detection efficiency is met at 15s for a 40m standoff, and 1.2s for a 20m standoff.

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LDRD Annual Report

Sweany, Melinda D.

This is a high-risk effort to leverage knowledge gained from previous work, which focused on detector development leading to better energy resolution and reconstruction errors. This work seeks to enable applications that require precise elemental characterization of materials, such as chemical munitions remediation, offering the potential to close current detection gaps.

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Enabling Explosives and Contraband Detection

Sweany, Melinda D.; Marleau, P.; Monterial, M.

We present the design and performance of a proof-of-concept 32 channel material identification system. Our system is based on the energy-dependent attenuation of fast neutrons for four elements: hydrogen, carbon, nitrogen and oxygen. We describe a new approach to obtaining a broad range of neutron energies to probe a sample, as well as our technique for reconstructing the molar densities within a sample. The system's performance as a function of time-of-flight energy resolution is explored using a Geant4-based Monte Carlo. Our results indicate that, with the expected detector response of our system, we will be able to determine the molar density of all four elements to within a 20-30% accuracy in a two hour scan time. In many cases this error is systematically low, thus the ratio between elements is more accurate. This degree of accuracy is enough to distinguish, for example, a sample of water from a sample of pure hydrogen peroxide: the ratio of oxygen to hydrogen is reconstructed to within 8 0.5% of the true value. Finally, with future algorithm development that accounts for backgrounds caused by scattering within the sample itself, the accuracy of molar densities, not ratios, may improve to the 5-10% level for a two hour scan time. Experimental performance was evaluated with various thicknesses of polyethylene. The detector response in terms of energy, particle identification, and timing are presented as well.

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Design and expected performance of a fast neutron attenuation probe for light element density measurements

Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment

Sweany, Melinda D.; Marleau, P.

We present the design and expected performance of a proof-of-concept 32 channel material identification system. Our system is based on the energy-dependent attenuation of fast neutrons for four elements: hydrogen, carbon, nitrogen and oxygen. We describe a new approach to obtaining a broad range of neutron energies to probe a sample, as well as our technique for reconstructing the molar densities within a sample. The system's performance as a function of time-of-flight energy resolution is explored using a Geant4-based Monte Carlo. Our results indicate that, with the expected detector response of our system, we will be able to determine the molar density of all four elements to within a 20–30% accuracy in a two hour scan time. In many cases this error is systematically low, thus the ratio between elements is more accurate. This degree of accuracy is enough to distinguish, for example, a sample of water from a sample of pure hydrogen peroxide: the ratio of oxygen to hydrogen is reconstructed to within 8±0.5% of the true value. Finally, with future algorithm development that accounts for backgrounds caused by scattering within the sample itself, the accuracy of molar densities, not ratios, may improve to the 5–10% level for a two hour scan time.

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Low light event reconstruction simulations for an optically segmented single volume scatter camera

2015 IEEE Nuclear Science Symposium and Medical Imaging Conference, NSS/MIC 2015

Weinfurther, Kyle; Mattingly, John; Brubaker, E.; Steele, J.; Sweany, Melinda D.; Braverman, Joshua

Dual plane neutron scatter cameras have shown promise for localizing fast neutron sources. The condition that a neutron must scatter in both planes of the camera produces low counting efficiencies. Counting efficiency can be improved using an alternative design that uses a single, optically segmented volume of scintillation material. Using Geant4, we simulated pulses from neutron elastic scatter events at different locations throughout an EJ-204 scintillator bar. We used nonlinear regression on low light pulses to determine the position along the bar where the scatter event occurred.

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Design of a transportable high efficiency fast neutron spectrometer

Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment

Roecker, C.; Bernstein, A.; Bowden, N.S.; Cabrera-Palmer, B.; Dazeley, S.; Gerling, Mark; Marleau, P.; Sweany, Melinda D.; Vetter, K.

A transportable fast neutron detection system has been designed and constructed for measuring neutron energy spectra and flux ranging from tens to hundreds of MeV. The transportability of the spectrometer reduces the detector-related systematic bias between different neutron spectra and flux measurements, which allows for the comparison of measurements above or below ground. The spectrometer will measure neutron fluxes that are of prohibitively low intensity compared to the site-specific background rates targeted by other transportable fast neutron detection systems. To measure low intensity high-energy neutron fluxes, a conventional capture-gating technique is used for measuring neutron energies above 20 MeV and a novel multiplicity technique is used for measuring neutron energies above 100 MeV. The spectrometer is composed of two Gd containing plastic scintillator detectors arranged around a lead spallation target. To calibrate and characterize the position dependent response of the spectrometer, a Monte Carlo model was developed and used in conjunction with experimental data from gamma ray sources. Multiplicity event identification algorithms were developed and used with a Cf-252 neutron multiplicity source to validate the Monte Carlo model Gd concentration and secondary neutron capture efficiency. The validated Monte Carlo model was used to predict an effective area for the multiplicity and capture gating analyses. For incident neutron energies between 100 MeV and 1000 MeV with an isotropic angular distribution, the multiplicity analysis predicted an effective area of 500 cm2 rising to 5000 cm2. For neutron energies above 20 MeV, the capture-gating analysis predicted an effective area between 1800 cm2 and 2500 cm2. The multiplicity mode was found to be sensitive to the incident neutron angular distribution.

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A search for cosmogenic production of β-neutron emitting radionuclides in water

Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment

Sweany, Melinda D.; Dazeley, S.; Askins, M.; Bergevin, M.; Bernstein, A.; Bowden, N.S.; Jaffke, P.; Rountree, S.D.; Shokair, T.M.

Here we present the first results of WATCHBOY, a water Cherenkov detector designed to measure the yield of β-neutron emitting radionuclides produced by cosmic ray muons in water. In addition to the β-neutron measurement, we also provide a first look at isolating single-β producing radionuclides following muon-induced hadronic showers as a check of the detection capabilities of WATCHBOY. The data taken over 207 live days indicates a 9Li production yield upper limit of 1.9× 10-7μ-1g-1 cm2 at ∼400 m water equivalent (m.w.e.) overburden at the 90% confidence level. In this work the 9Li signal in WATCHBOY was used as a proxy for the combined search for 9Li and 8He production. This result will provide a constraint on estimates of antineutrino-like backgrounds in future water-based antineutrino detectors.

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Demonstration of two-dimensional time-encoded imaging of fast neutrons

Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment

Sweany, Melinda D.; Brubaker, E.; Gerling, Mark; Le Galloudec, Nathalie J.; Marleau, P.; Mcmillan, K.; Nowack, A.; Brennan, J.

We present a neutron detector system based on time-encoded imaging, and demonstrate its applicability toward the spatial mapping of special nuclear material. We demonstrate that two-dimensional fast-neutron imaging with 2° resolution at 2 m stand-off is feasible with only two instrumented detectors.

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Enabling Explosives and Contraband Detection with Neutron Resonant Attenuation. Year 1 of 3 Summary

Sweany, Melinda D.

Material Identification by Resonant Attenuation is a technique that measures the energy-dependent attenuation of 1-10 MeV neutrons as they pass through a sample. Elemental information is determined from the neutron absorption resonances unique to each element. With sufficient energy resolution, these resonances can be used to categorize a wide range of materials, serving as a powerful discrimination technique between explosives, contraband, and other materials. Our proposed system is unique in that it simultaneously down-scatters and time tags neutrons in scintillator detectors oriented between a d-T generator and sample. This allows not only for energy measurements without pulsed neutron beams, but for sample interrogation over a large range of relevant energies, vastly improving scan times. Our system’s core advantage is a potential breakthrough ability to provide detection discrimination of threat materials by their elemental composition (e.g. water vs. hydrogen peroxide) without opening the container. However, several technical and computational challenges associated with this technique have yet to be addressed. There are several open questions: what is the sensitivity to different materials, what scan times are necessary, what are the sources of background, how do each of these scale as the detector system is made larger, and how can the system be integrated into existing scanning technology to close current detection gaps? In order to prove the applicability of this technology, we will develop a validated model to optimize the design and characterize the uncertainties in the measurement, and then test the system in a real-world scenario. This project seeks to perform R&D and laboratory tests that demonstrate proof of concept (TRL 3) to establishing an integrated system and evaluating its performance (TRL 4) through both laboratory tests and a validated detector model. The validated model will allow us to explore our technology’s benefits to explosive detection in various applications.

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Preliminary study of the inclusion of Water-based Liquid Scintillator in the WATCHMAN Detector

Sweany, Melinda D.; Feng, Patrick L.; Marleau, P.

This note summarizes an effort to characterize the effects of adding water-based liquid scintillator to the WATCHMAN detector. A detector model was built in the Geant4 Monte Carlo toolkit, and the position reconstruction of positrons within the detector was compared with and without scintillator. This study highlights the need for further modeling studies and small-scale experimental studies before inclusion into a large-scale detector, as the benefits compared to the associated costs are unclear.

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Multi-depth Measurement of Fast Neutrons

Marleau, P.; Gerling, Mark; Sweany, Melinda D.; Cabrera-Palmer, B.; Brennan, J.

A spallation based multiplicity detector has been constructed and deployed to the Kimballton Underground Research Facility to measure the cosmogenic fast neutron flux anti-coincident from the initiating muon. Two of the three planned measurements have been completed (~380 and ~600 m.w.e) with sufficient statistics. The third measurement at level 14 (~4450 m.w.e.) is currently being performed. Current results at ~600 m.w.e. compare favourably to the one previous measurement at 550 m.w.e. For neutron energies between 100 and 200 MeV measurements at ~380 m.w.e. produce fluxes between 1e-8 and 7e-9 n/cm2/s/MeV and at ~600 m.w.e. measurements produce fluxes between 7e-9 and 1e-11 n/cm2/s/MeV.

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Above-ground Antineutrino Detection for Nuclear Reactor Monitoring

Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment

Sweany, Melinda D.; Brennan, J.; Cabrera-Palmer, B.; Kiff, Scott; Reyna, David R.; Throckmorton, Daniel J.

Antineutrino monitoring of nuclear reactors has been demonstrated many times, however the technique has not as of yet been developed into a useful capability for treaty verification purposes. The most notable drawback is the current requirement that detectors be deployed underground, with at least several meters-water-equivalent of shielding from cosmic radiation. In addition, the deployment of liquid-based detector media presents a challenge in reactor facilities. We are currently developing a detector system that has the potential to operate above ground and circumvent deployment problems associated with a liquid detection media: the system is composed of segments of plastic scintillator surrounded by 6LiF/ZnS:Ag. ZnS:Ag is a radio-luminescent phosphor used to detect the neutron capture products of lithium-6. Because of its long decay time compared to standard plastic scintillators, pulse-shape discrimination can be used to distinguish positron and neutron interactions resulting from the inverse beta decay (IBD) of antineutrinos within the detector volume, reducing both accidental and correlated backgrounds. Segmentation further reduces backgrounds by identifying the positron’s annihilation gammas, which are absent for most correlated and uncorrelated backgrounds. This work explores different configurations in order to maximize the size of the detector segments without reducing the intrinsic neutron detection efficiency. We believe this technology will ultimately be applicable to potential safeguards scenarios such as those recently described.

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Bubble masks for time-encoded imaging of fast neutrons

Brubaker, E.; Brennan, J.; Marleau, P.; Steele, J.; Sweany, Melinda D.; Throckmorton, Daniel J.

Time-encoded imaging is an approach to directional radiation detection that is being developed at SNL with a focus on fast neutron directional detection. In this technique, a time modulation of a detected neutron signal is inducedtypically, a moving mask that attenuates neutrons with a time structure that depends on the source position. An important challenge in time-encoded imaging is to develop high-resolution two-dimensional imaging capabilities; building a mechanically moving high-resolution mask presents challenges both theoretical and technical. We have investigated an alternative to mechanical masks that replaces the solid mask with a liquid such as mineral oil. Instead of fixed blocks of solid material that move in pre-defined patterns, the oil is contained in tubing structures, and carefully introduced air gapsbubblespropagate through the tubing, generating moving patterns of oil mask elements and air apertures. Compared to current moving-mask techniques, the bubble mask is simple, since mechanical motion is replaced by gravity-driven bubble propagation; it is flexible, since arbitrary bubble patterns can be generated by a software-controlled valve actuator; and it is potentially high performance, since the tubing and bubble size can be tuned for high-resolution imaging requirements. We have built and tested various single-tube mask elements, and will present results on bubble introduction and propagation as a function of tubing size and cross-sectional shape; real-time bubble position tracking; neutron source imaging tests; and reconstruction techniques demonstrated on simple test data as well as a simulated full detector system.

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Bubble masks for time-encoded imaging of fast neutrons

IEEE Nuclear Science Symposium Conference Record

Brubaker, E.; Brennan, J.; Steele, J.; Sweany, Melinda D.; Throckmorton, Daniel J.

Time-encoded imaging is an approach to directional radiation detection that is being developed at SNL with a focus on fast neutron directional detection. In this technique, a time modulation of a detected neutron signal is induced - typically, a moving mask that attenuates neutrons with a time structure that depends on the source position. An important challenge in time-encoded imaging is to develop high-resolution two-dimensional imaging capabilities; building a mechanically moving high-resolution mask presents challenges both theoretical and technical. We have investigated an alternative to mechanical masks that replaces the solid mask with a liquid such as mineral oil. Instead of fixed blocks of solid material that move in predefined patterns, the oil is contained in tubing structures, and carefully introduced air gaps - bubbles - propagate through the tubing, generating moving patterns of oil mask elements and air apertures. Compared to current moving-mask techniques, the bubble mask is simple, since mechanical motion is replaced by gravity-driven bubble propagation; it is flexible, since arbitrary bubble patterns can be generated by a software-controlled valve actuator; and it is potentially high performance, since the tubing and bubble size can be tuned for high-resolution imaging requirements. We have built and tested various single-tube mask elements, and will present results on bubble introduction and propagation for different tube sizes and cross-sectional shapes; real-time bubble position tracking; neutron source imaging tests; and reconstruction techniques demonstrated on simple test data as well as a simulated full detector system. © 2013 IEEE.

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Bubble masks for time-encoded imaging of fast neutrons

IEEE Nuclear Science Symposium Conference Record

Brennan, J.; Brubaker, E.; Steele, J.; Sweany, Melinda D.; Throckmorton, Daniel J.

Time-encoded imaging is an approach to directional radiation detection that is being developed at SNL with a focus on fast neutron directional detection. In this technique, a time modulation of a detected neutron signal is induced - typically, a moving mask that attenuates neutrons with a time structure that depends on the source position. An important challenge in time-encoded imaging is to develop high-resolution two-dimensional imaging capabilities; building a mechanically moving high-resolution mask presents challenges both theoretical and technical. We have investigated an alternative to mechanical masks that replaces the solid mask with a liquid such as mineral oil. Instead of fixed blocks of solid material that move in predefined patterns, the oil is contained in tubing structures, and carefully introduced air gaps - bubbles - propagate through the tubing, generating moving patterns of oil mask elements and air apertures. Compared to current moving-mask techniques, the bubble mask is simple, since mechanical motion is replaced by gravity-driven bubble propagation; it is flexible, since arbitrary bubble patterns can be generated by a software-controlled valve actuator; and it is potentially high performance, since the tubing and bubble size can be tuned for high-resolution imaging requirements. We have built and tested various single-tube mask elements, and will present results on bubble introduction and propagation for different tube sizes and cross-sectional shapes; real-time bubble position tracking; neutron source imaging tests; and reconstruction techniques demonstrated on simple test data as well as a simulated full detector system. © 2013 IEEE.

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79 Results