Publications

Abstract not provided.

At the Z Facility at Sandia National Laboratories, the magnetized liner inertial fusion (MagLIF) program aims to study the inertial confinement fusion in deuterium-filled gas cells by implementing a three-step process on the fuel: premagnetization, laser preheat, and Z-pinch compression. In the laser preheat stage, the Z-Beamlet laser focuses through a thin polyimide window to enter the gas cell and heat the fusion fuel. However, it is known that the presence of the few μm thick window reduces the amount of laser energy that enters the gas and causes window material to mix into the fuel. These effects are detrimental to achieving fusion; therefore, a windowless target is desired. The Lasergate concept is designed to accomplish this by "cutting"the window and allowing the interior gas pressure to push the window material out of the beam path just before the heating laser arrives. In this work, we present the proof-of-principle experiments to evaluate a laser-cutting approach to Lasergate and explore the subsequent window and gas dynamics. Further, an experimental comparison of gas preheat with and without Lasergate gives clear indications of an energy deposition advantage using the Lasergate concept, as well as other observed and hypothesized benefits. While Lasergate was conceived with MagLIF in mind, the method is applicable to any laser or diagnostic application requiring direct line of sight to the interior of gas cell targets.

Abstract not provided.

Abstract not provided.

Abstract not provided.

Abstract not provided.

Abstract not provided.

Abstract not provided.

Abstract not provided.

Abstract not provided.

Dichroic coatings have been developed for high transmission at 527 nm and high reflection at 1054 nm for laser operations in the nanosecond pulse regime. The coatings consist of HfO2 and SiO2 layers deposited with e-beam evaporation, and laser-induced damage thresholds as high as 12.5 J/cm2 were measured at 532 nm with 3.5 ns pulses (22.5 degrees angle of incidence, in S-polarization). However, laser damage measurements at the single wavelength of 532 nm do not adequately characterize the laser damage resistance of these coatings, since they were designed to operate at dual wavelengths simultaneously. This became apparent after one of the coatings damaged prematurely at a lower fluence in the beam train, which inspired further investigations. To gain a more complete understanding of the laser damage resistance, results of a dual-wavelength laser damage test performed at both 532 nm and 1064 nm are presented.

Abstract not provided.

Abstract not provided.

X-ray diffraction measurements to characterize phase transitions of dynamically compressed high-Z matter at Mbar pressures require both sufficient photon energy and fluence to create data with high fidelity in a single shot. Large-scale laser systems can be used to generate x-ray sources above 10 keV utilizing line radiation of mid-Z elements. However, the laser-to-x-ray energy conversion efficiency at these energies is low, and thermal x-rays or hot electrons result in unwanted background. We employ polycapillary x-ray lenses in powder x-ray diffraction measurements using solid target x-ray emission from either the Z-Beamlet long-pulse or the Z-Petawatt (ZPW) short-pulse laser systems at Sandia National Laboratories. Polycapillary lenses allow for a 100-fold fluence increase compared to a conventional pinhole aperture while simultaneously reducing the background significantly. This enables diffraction measurements up to 16 keV at the few-photon signal level as well as diffraction experiments with ZPW at full intensity.

Abstract not provided.

Abstract not provided.

Existing models for most materials do not describe phase transformations and associated lattice dy- namics (kinetics) under extreme conditions of pressure and temperature. Dynamic x-ray diffraction (DXRD) allows material investigations in situ on an atomic scale due to the correlation between solid-state structures and their associated diffraction patterns. In this LDRD project we have devel- oped a nanosecond laser-compression and picosecond-to-nanosecond x-ray diffraction platform for dynamically-compressed material studies. A new target chamber in the Target Bay in building 983 was commissioned for the ns, kJ Z-Beamlet laser (ZBL) and the 0.1 ns, 250 J Z-Petawatt (ZPW) laser systems, which were used to create 8-16 keV plasma x-ray sources from thin metal foils. The 5 ns, 15 J Chaco laser system was converted to a high-energy laser shock driver to load material samples to GPa stresses. Since laser-to-x-ray energy conversion efficiency above 10 keV is low, we employed polycapillary x-ray lenses for a 100-fold fluence increase compared to a conventional pinhole aperture while simultaneously reducing the background significantly. Polycapillary lenses enabled diffraction measurements up to 16 keV with ZBL as well as diffraction experiments with ZPW. This x-ray diffraction platform supports experiments that are complementary to gas guns and the Z facility due to different strain rates. Ultimately, there is now a foundation to evaluate DXRD techniques and detectors in-house before transferring the technology to Z. This page intentionally left blank.

Abstract not provided.

Abstract not provided.

We report on progress for increasing the laser-induced damage threshold of dichroic beam combiner coatings for high transmission at 527 nm and high reflection at 1054 nm (22.5° angle of incidence, S-polarization). The initial coating consisted of HfO2 and SiO2 layers deposited with electron beam evaporation, and the laser-induced damage threshold was 7 J/cm2 at 532 nm with 3.5 ns pulses. This study introduces different coating strategies that were utilized to increase the laser damage threshold of this coating to 12.5 J/cm2.

Abstract not provided.

Abstract not provided.

Abstract not provided.

We designed an optical coating based on TiO2/SiO2 layer pairs for broad bandwidth high reflection (BBHR) at 45-deg angle of incidence (AOI), P polarization of femtosecond (fs) laser pulses of 900-nm center wavelength, and produced the coatings in Sandia's large optics coater by reactive, ion-assisted e-beam evaporation. This paper reports on laser-induced damage threshold (LIDT) tests of these coatings. The broad HR bands of BBHR coatings pose challenges to LIDT tests. An ideal test would be in a vacuum environment appropriate to a high energy, fs-pulse, petawatt-class laser, with pulses identical to its fs pulses. Short of this would be tests over portions of the HR band using nanosecond or sub-picosecond pulses produced by tunable lasers. Such tests could, e.g., sample 10-nm-wide wavelength intervals with center wavelengths tunable over the broad HR band. Alternatively, the coating's HR band could be adjusted by means of wavelength shifts due to changing the AOI of the LIDT tests or due to the coating absorbing moisture under ambient conditions. We had LIDT tests performed on the BBHR coatings at selected AOIs to gain insight into their laser damage properties and analyze how the results of the different LIDT tests compare.

We designed and produced optical coatings for broad bandwidth high reflection (BBHR) of femtosecond (fs) pulses for high energy petawatt (PW) lasers. These BBHR coatings consist of TiO2/SiO2 and/or HfO2/SiO2 layer pairs formed by reactive E-beam evaporation with ion-assisted deposition in Sandia's Large Optics Coating Facility. Specifications for the HR band and center wavelength of the coatings are for 45° angle of incidence (AOI), P polarization (Ppol), with use of the coatings at different AOIs and in humid or dry/vacuum environments providing corresponding different HR center wavelengths and spectral widths. These coatings must provide high laserinduced damage threshold (LIDT) to handle the PW fluences, and also low group delay dispersion (GDD) to reflect fs pulses without distortion of their temporal profiles. We present results of LIDT and GDD measurements on these coatings. The LIDT tests are at 45° or 65° AOI, Ppol in a dry environment with 100 fs laser pulses of 800 nm line center for BBHR coatings whose HR band line centers are near 800 nm. A GDD measurement for one of the BBHR coatings whose design HR center wavelength is near 900 nm shows reasonably low and smoothly varying GDD over the HR band. Our investigations include BBHR coatings designed for 45° AOI, Ppol with HR bands centered at 800 nm in dry or vacuum environments, and featuring three options: all TiO2/SiO2 layer pairs; all HfO2/SiO2 layer pairs; and TiO2/SiO2 inner layer pairs with 5 outer HfO2/SiO2 layer pairs. LIDT tests of these coatings with 100 fs, 800 nm line center pulses in their use environment show that replacing a few outer TiO2 layers of TiO2/SiO2 BBHR coatings with HfO2 leads to ∼ 80% higher LIDT with only minor loss of HR bandwidth.