Publications
Development of Elastic Recoil Detection Technique for Quantifying Light Isotope Concentrations in Irradiated TPBAR Materials
Doyle, Barney L.; Taylor, Caitlin A.; Hattar, Khalid M.; Muntifering, Brittany R.
The National Nuclear Security Administration's Tritium Sustainment Program is responsible for the design, development, demonstration, testing, analysis, and characterization of tritium-producing burnable absorber rods (TPBARs) and their components, in addition to producing tritium for the nation's strategic stockpile. The FY18 call for proposals included the specific basic science research topic, "Demonstration and evaluation of advanced characterization methods, particularly for quantifying the concentration of light isotopes (1H, 2H, and 4He, 6Li, and 7Li) in metal or ceramic matrices". A project IWO-389859 was awarded to the Ion Beam Lab (IBL) at Sandia-NM in FY18. This reports the success we had in developing and demonstrating such a method: 42 MeV Si+ 7 from the IBL' s Tandem was used to recoil these light isotopes into special detectors that separated all these isotopes by simultaneously measuring the energy and stopping power of these reoils. This technique, called Heavy Ion - Elastic Recoil Detection or HI-ERD, accurately measured the enriched 6 Li/Li-total of 0.246 +- 0.016, compared to the known value of 0.239. The isotopes 1H, 2H, 4He, 6Li and 7Li were also measured. (page intentionally left blank)