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Publications / Journal Article

3D strain-induced superconductivity in La2CuO4+δ using a simple vertically aligned nanocomposite approach

Choi, Eun M.; Di Bernardo, Angelo; Zhu, Bonan; Lu, Ping L.; Alpern, Hen; Zhang, Kelvin H.L.; Shapira, Tamar; Feighan, John; Lu, Ping L.; Robinson, Jason; Paltiel, Yossi; Millo, Oded; Wang, Haiyan; Jia, Quanxi; MacManus-Driscoll, Judith L.

A long-term goal for superconductors is to increase the superconducting transition temperature, TC. In cuprates, TC depends strongly on the out-of-plane Cu-apical oxygen distance and the in-plane Cu-O distance, but there has been little attention paid to tuning them independently. Here, in simply grown, self-assembled, vertically aligned nanocomposite thin films of La2CuO4+δ + LaCuO3, by strongly increasing out-of-plane distances without reducing in-plane distances (three-dimensional strain engineering), we achieve superconductivity up to 50 K in the vertical interface regions, spaced ∼50 nm apart. No additional process to supply excess oxygen, e.g., by ozone or high-pressure oxygen annealing, was required, as is normally the case for plain La2CuO4+δ films. Our proof-of-concept work represents an entirely new approach to increasing TC in cuprates or other superconductors.